Raman spectroscopic measurements of (1) band of hydrogen sulfide over a wide range of temperature and density in fused-silica optical cells
Jiang, Lei1; Xin, Yang1,2; Chou, I-Ming1; Chen, Ying1; Jiang, Lei(Chinese Acad Sci, Inst Deep Sea Sci & Engn, CAS Key Lab Expt Study Deep Sea Extreme Condit, Sanya 572000, Hainan, Peoples R China); Chou, I-Ming(Chinese Acad Sci, Inst Deep Sea Sci & Engn, CAS Key Lab Expt Study Deep Sea Extreme Condit, Sanya 572000, Hainan, Peoples R China)
2018-02-01
发表期刊JOURNAL OF RAMAN SPECTROSCOPY
卷号49期号:2页码:343-350
产权排序第1完成单位 ; 第2完成单位
摘要A method was developed to determine the fluid density of pure hydrogen sulfide (H2S) at a fixed temperature using Raman spectroscopic measurements. The positions of the H2S Raman (1) band were measured at a wide range of temperatures (188.15KT633.15K) and pressures (P506bar) using fused-silica capillary capsules and high-pressure optical cells. The relation among H2S density (), H2S (1) peak position, and T can be represented by =2447.680+0.127xT-1.876x(1)-0.000001xT(2)-0.000048x Tx(1)+0.00036x(1)(2) (root-mean-square error=0.0197g/cm(3) and correlation coefficient=0.9963). This equation can be applied to calculate the density of the H2S fluid from the measured H2S (1) peak position at a given temperature. Finally, the effects of temperature and H2S density on (1) peak position were examined using isochoric and isothermal experiments.
文章类型Article
关键词Density Fused-silica Optical Cells Hydrogen Sulfide Raman Spectroscopy Temperature
WOS标题词Science & Technology ; Technology
DOI10.1002/jrs.5293
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收录类别SCI
语种英语
关键词[WOS]HIGH-PRESSURE PHASE ; FLUID INCLUSIONS ; CARBON-DIOXIDE ; LIQUID-STATE ; NATURAL-GAS ; H2S ; CO2 ; CALIBRATION ; SPECTRA ; WATER
WOS类目Spectroscopy
WOS记录号WOS:000425020500017
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文献类型期刊论文
条目标识符http://ir.idsse.ac.cn/handle/183446/5925
专题深海科学研究部_深海极端环境模拟研究实验室
通讯作者Jiang, Lei; Chou, I-Ming; Jiang, Lei(Chinese Acad Sci, Inst Deep Sea Sci & Engn, CAS Key Lab Expt Study Deep Sea Extreme Condit, Sanya 572000, Hainan, Peoples R China); Chou, I-Ming(Chinese Acad Sci, Inst Deep Sea Sci & Engn, CAS Key Lab Expt Study Deep Sea Extreme Condit, Sanya 572000, Hainan, Peoples R China)
作者单位1.Chinese Acad Sci, Inst Deep Sea Sci & Engn, CAS Key Lab Expt Study Deep Sea Extreme Condit, Sanya 572000, Hainan, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
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Jiang, Lei,Xin, Yang,Chou, I-Ming,et al. Raman spectroscopic measurements of (1) band of hydrogen sulfide over a wide range of temperature and density in fused-silica optical cells[J]. JOURNAL OF RAMAN SPECTROSCOPY,2018,49(2):343-350.
APA Jiang, Lei,Xin, Yang,Chou, I-Ming,Chen, Ying,Jiang, Lei,&Chou, I-Ming.(2018).Raman spectroscopic measurements of (1) band of hydrogen sulfide over a wide range of temperature and density in fused-silica optical cells.JOURNAL OF RAMAN SPECTROSCOPY,49(2),343-350.
MLA Jiang, Lei,et al."Raman spectroscopic measurements of (1) band of hydrogen sulfide over a wide range of temperature and density in fused-silica optical cells".JOURNAL OF RAMAN SPECTROSCOPY 49.2(2018):343-350.
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